Ex parte ROSS et al. - Page 6




          Appeal No. 95-0432                                                           
          Application 08/002,448                                                       
                    The present invention provides techniques, methods,                
               and additive combinations which permit the integral                     
               blending of additives for filler/polymer composites for                 
               the enhancement of physical properties such as impact                   
               strength, tensile strength, etc.  The present invention                 
               provides novel methods for reinforcing thermoplastic                    
               organic polymers such as polyethylene and polypropylene                 
               by blending the polymer, a finely divided filler and a                  
               surfactant which is a siloxane-polyoxyalkylene block                    
               copolymer or a siloxane containing at least one silicone                
               bonded alkyl group of 12 or more carbon atoms or a                      
               polyoxyalkylene compound containing polyoxyalkylene                     
               blocks terminated at one end by an alkyl group having 12                
               or more carbon atoms or an alkenyl group and terminated                 
               at the other end by an alkoxy group or a hydroxy group.                 
               According to this invention, the novel method also                      
          includes                                                                     
               the incorporation of an unsaturated silicon compound                    
               containing at least one polymerizable unsaturated group,                
               at least one /SiO-group and not more than 5 silicon                     
          atoms,                                                                       
               e.g. a polymerizable unsaturated hydrolyzable silane                    
               coupling agent and/or an unsaturated organic compound                   
               containing two or more polymerizable unsaturated groups                 
               into the filler/-polymer mixture to provide synergistic                 
               enhancement of the filled polymer physical properties.                  
               The surfactants Godlewski prefers are polysiloxane-                     
          polyalkyleneoxyalkylene block copolymers (col. 6, l. 38-39).                 
          Nevertheless, Godlewski teaches that polysiloxane-polyalkylene               
          block copolymer surfactants, i.e., siloxanes containing at                   
          least one silicon bonded alkyl group of 12 or more carbon                    
          atoms,                                                                       
          are useful in the invention (col. 5, l. 31-45).  At column 6,                
          line 57, to column 7, line 13, Godlewski lists polymeric                     

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