GALIMBERTI et al. V. ASANUMA et al. - Page 2




                 Interference No. 103,303                                                                                                               



                 RONALD H. SMITH, SOFOCLEOUS and HANLON, Administrative Patent                                                                          
                 Judges.                                                                                                                                
                 SOFOCLEOUS, Administrative Patent Judge.                                                                                               
                                                               FINAL DECISION                                                                           
                          The subject matter of this interference relates to                                                                            
                 crystalline copolymers of propylene and 1-butene and a process                                                                         
                 for preparing the copolymers.  The counts of this interference                                                                         
                 are as follows:                                                                                                                        
                 Count 1                                                                                                                                
                          Crystalline copolymers of propylene and 1-butene with an                                                                      
                 essentially syndiotactic structure, containing from 1.3 to                                                                             
                 10 mole % of 1-butene units, having a melting point from 110E                                                                          
                 to 140EC., a fraction soluble in xylene at 25EC. less than 10%                                                                         
                 by weight, and a composition similar to the mixture of the                                                                             
                 monomers present in the gas phase during preparation of said                                                                           
                 polymer, wherein the difference between the amount of                                                                                  
                 comonomer present in the gas phase and the amount of comonomer                                                                         
                 in said composition is between 13% to 23% less in the                                                                                  
                 composition of said copolymer;                                                                                                         
                                                                          or                                                                            
                 a syndiotactic propylene copolymer comprising 76 to 99 mole %                                                                          
                 of propylene and 1 to 24 mole percent of butene wherein in the                                                                         
                 13C-NMR spectrum of said syndiotactic propylene copolymer, said                                                                        
                 copolymer exhibits a ratio of the intensity of a peak at about                                                                         
                 20.2 ppm to the sum of the intensities of the total peaks                                                                              
                 attributable to methyl groups in propylene units at about 19-                                                                          
                 22 of 0.5 or more.                                                                                                                     
                 Count 2                                                                                                                                
                          A process for the preparation of the copolymers of count 1                                                                    
                 comprising the polymerization of gaseous mixtures of propylene                                                                         

                                                                          -2-                                                                           




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